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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ANGEO</journal-id><journal-title-group>
    <journal-title>Annales Geophysicae</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ANGEO</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Ann. Geophys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1432-0576</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/angeo-36-321-2018</article-id><title-group><article-title>Aerosol indirect effects on summer precipitation in a regional climate model for the Euro-Mediterranean region</article-title><alt-title>Aerosol indirect effects on summer precipitation in the Euro-Mediterranean region</alt-title>
      </title-group><?xmltex \runningtitle{Aerosol indirect effects on summer precipitation in the Euro-Mediterranean region}?><?xmltex \runningauthor{N. Da Silva et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Da Silva</surname><given-names>Nicolas</given-names></name>
          <email>nicolas.da-silva@lmd.polytechnique.fr</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff2">
          <name><surname>Mailler</surname><given-names>Sylvain</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Drobinski</surname><given-names>Philippe</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>LMD/IPSL, École polytechnique, Université Paris Saclay, ENS, PSL Research University, Sorbonne Universités,<?xmltex \hack{\newline}?>
UPMC Univ Paris 06, CNRS, Palaiseau, France</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>École des Ponts ParisTech, Université Paris-Est, 77455 Champs-sur-Marne,
France</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Nicolas Da Silva (nicolas.da-silva@lmd.polytechnique.fr)</corresp></author-notes><pub-date><day>6</day><month>March</month><year>2018</year></pub-date>
      
      <volume>36</volume>
      <issue>2</issue>
      <fpage>321</fpage><lpage>335</lpage>
      <history>
        <date date-type="received"><day>31</day><month>October</month><year>2017</year></date>
           <date date-type="rev-recd"><day>24</day><month>January</month><year>2018</year></date>
           <date date-type="accepted"><day>25</day><month>January</month><year>2018</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2018 Nicolas Da Silva et al.</copyright-statement>
        <copyright-year>2018</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018.html">This article is available from https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018.html</self-uri><self-uri xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018.pdf">The full text article is available as a PDF file from https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018.pdf</self-uri>
      <abstract>
    <p id="d1e106">Aerosols affect atmospheric dynamics through their direct and
semi-direct effects as well as through their effects on cloud microphysics
(indirect effects). The present study investigates the indirect effects of
aerosols on summer precipitation in the Euro-Mediterranean region, which is
located at the crossroads of air masses carrying both natural and
anthropogenic aerosols. While it is difficult to disentangle the indirect
effects of aerosols from the direct and semi-direct effects in reality, a
numerical sensitivity experiment is carried out using the Weather Research
and Forecasting (WRF) model, which allows us to isolate indirect effects, all
other effects being equal. The Mediterranean hydrological cycle has often
been studied using regional climate model (RCM) simulations with
parameterized convection, which is the approach we adopt in the present
study. For this purpose, the Thompson aerosol-aware microphysics scheme is
used in a pair of simulations run at 50 km resolution with extremely high
and low aerosol concentrations.
An additional pair of simulations has been
performed at a convection-permitting resolution (3.3 km) to examine these
effects without the use of parameterized convection.</p>
    <p id="d1e109">While the reduced radiative flux due to the direct effects of the aerosols is
already known to reduce precipitation amounts, there is still no general
agreement on the sign and magnitude of the aerosol indirect
forcing effect on precipitation,
with various processes competing with each other. Although some processes
tend to enhance precipitation amounts, some others tend to reduce them. In
these simulations, increased aerosol loads lead to weaker precipitation in
the parameterized (low-resolution) configuration. The fact that a similar
result is obtained for a selected area in the convection-permitting
(high-resolution) configuration allows for physical interpretations. By
examining the key variables in the model outputs, we propose a causal chain
that links the aerosol effects on microphysics to their simulated effect on
precipitation, essentially through reduction of the radiative heating of the
surface and corresponding reductions of surface temperature, resulting in
increased atmospheric stability in the presence of high aerosol loads.</p>
  </abstract>
      <kwd-group>
        <kwd>Atmospheric composition and structure (aerosols and particles)</kwd>
      </kwd-group>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p id="d1e119">The hydrological cycle in the Mediterranean is a key environmental and
socioeconomic question for a wide region including southern Europe, northern
Africa, and the Middle East <xref ref-type="bibr" rid="bib1.bibx12" id="paren.1"/>. The Mediterranean climate is
characterized by hot summers and mild winters, and by the fact that
wintertime is much more rainy than summertime. Historically, it has been
proposed to define the Mediterranean climate by the criterion that wintertime
precipitation total exceeds 3 times the summertime precipitation total
<xref ref-type="bibr" rid="bib1.bibx27" id="paren.2"/>. <xref ref-type="bibr" rid="bib1.bibx78" id="normal.3"/> show that wintertime precipitation
accounts for at least 50–60 % of the total annual rainfall in the western and
northern parts of the Mediterranean basin and up to 70–90 % in the
southern and eastern parts.</p>
      <p id="d1e131">There is a need for better understanding precipitation variability, including
intensity and frequency, in the Mediterranean region. This is one of the main
objectives of the HyMeX (Hydrological cycle in the Mediterranean Experiment)
international program <xref ref-type="bibr" rid="bib1.bibx12" id="paren.4"/>.<?pagebreak page322?> Regional climate models (RCMs) have
frequently been used for that purpose
<xref ref-type="bibr" rid="bib1.bibx33 bib1.bibx67 bib1.bibx19 bib1.bibx6 bib1.bibx13 bib1.bibx14" id="paren.5"/> with
horizontal scales ranging from 20 to 50 km and parameterized convection.
While direct effects of aerosol have already been examined on the regional
scale over the Mediterranean <xref ref-type="bibr" rid="bib1.bibx41 bib1.bibx42" id="paren.6"/>, these simulations do
not usually take into account the indirect effects of aerosols. Therefore,
the present study aims at exploring the possible impacts of aerosol indirect
effects in such models on precipitation over that region. For that purpose,
we perform a pair of simulations using the WRF (weather research and
forecasting model version 3.7.1; <xref ref-type="bibr" rid="bib1.bibx65" id="altparen.7"/>) at a 50 km resolution
which is within the range of the typical long-term regional climate
simulations, with the <xref ref-type="bibr" rid="bib1.bibx24" id="normal.8"/> convection scheme and the
<xref ref-type="bibr" rid="bib1.bibx73" id="normal.9"/> aerosol-aware microphysics. One simulation is forced with
extremely strong concentrations of cloud condensation nuclei (CCN), and the
other one with extremely low concentrations. The use of this configuration
permits us to disconnect the direct effect of the aerosols from their indirect
effect, thereby isolating the indirect effect of aerosols on precipitation in
a RCM for the Mediterranean area. The processes governing precipitation
occurrence markedly differ between wintertime and summertime: while
large-scale stratiform precipitation largely dominates wintertime
precipitation, the contribution of small-scale convective precipitation is
significant in summertime. Therefore, restricting the focus of the study to
summertime precipitation permits us to examine in a more detailed way the
processes and causal chains by which the indirect effect of the aerosols
affect precipitation, allowing to examine both large-scale and parameterized
precipitation. As the representation of precipitation in RCMs is very
sensitive to the choice of the convection scheme <xref ref-type="bibr" rid="bib1.bibx10" id="paren.10"/>, and also
because it has been found that the use of parameterized convection might
hinder the correct representation of the microphysical effects of the
aerosols <xref ref-type="bibr" rid="bib1.bibx25" id="paren.11"/>, two additional simulations for a smaller domain at
a convection-permitting resolution (3.3 km) have been performed (HR for high
resolution). These two simulations
allow us to check that the effects observed in the two low resolution (LR)
simulations are not mere artifacts of the convection scheme, and also to
examine how the aerosol indirect effect affects summertime precipitation in a
convection-permitting model.</p>
      <p id="d1e159">The Mediterranean area is an area in which it is particularly important to
include all aerosol effects in RCM studies because it is located at the
crossroads of air masses carrying strong concentrations of both natural and
anthropogenic aerosols <xref ref-type="bibr" rid="bib1.bibx29 bib1.bibx55" id="paren.12"/>. Natural sources are mineral
dust from arid areas, secondary organic aerosols due to biogenic emissions,
biomass burning, volcanic emissions, and sea-salt emissions. Anthropogenic
sources are mainly due to fossil fuel burning by industrial facilities, power
plants, vehicles, and ships, as well as agricultural processes
<xref ref-type="bibr" rid="bib1.bibx51" id="paren.13"/>.</p>
      <p id="d1e168">Apart from their direct radiative effect
<xref ref-type="bibr" rid="bib1.bibx61 bib1.bibx39 bib1.bibx34 bib1.bibx71 bib1.bibx40" id="paren.14"/>, interactions between aerosols
and cloud water and ice occur through several processes. Aerosols act as
nuclei for the formation of cloud water and ice, changing the number and size
of the cloud droplets and ice particles, which affects the atmospheric
physics and dynamics in several ways. Aerosols have been hypothesized to
increase the liquid water content, the lifetime of clouds, and cloud height
through a decrease in droplet radius and the corresponding decrease of the
precipitation efficiency <xref ref-type="bibr" rid="bib1.bibx8 bib1.bibx52 bib1.bibx50 bib1.bibx57" id="paren.15"/>, an
effect often called the Albrecht effect <xref ref-type="bibr" rid="bib1.bibx2" id="paren.16"/>. However, recent
studies suggest that the Albrecht effect on liquid water content could be
compensated by enhanced evaporation and dry air entrainment
(<xref ref-type="bibr" rid="bib1.bibx66 bib1.bibx63" id="altparen.17"/>). Such an effect may depend on cloud types and
properties <xref ref-type="bibr" rid="bib1.bibx18" id="paren.18"/> and on the microphysics scheme <xref ref-type="bibr" rid="bib1.bibx79" id="paren.19"/>.
Another process known as the Twomey effect refers to increased cloud optical
depth (COD) with increased aerosol concentrations due to the diminished
droplet radius and increased droplet number <xref ref-type="bibr" rid="bib1.bibx74" id="paren.20"/>. Under certain
conditions, aerosols may also invigorate deep convective clouds by increasing
the release of latent energy <xref ref-type="bibr" rid="bib1.bibx58" id="paren.21"/>.</p>
      <p id="d1e197">Indirect effects are not as well understood as direct effects because many
different physical processes are involved and partly compensate each other
<xref ref-type="bibr" rid="bib1.bibx70" id="paren.22"/>. The buffered characteristic of clouds has been diagnosed
in several aerosol indirect effect studies
<xref ref-type="bibr" rid="bib1.bibx17 bib1.bibx20 bib1.bibx38 bib1.bibx62 bib1.bibx76" id="paren.23"/>. In numerical
simulation, <xref ref-type="bibr" rid="bib1.bibx62" id="normal.24"/> observed compensations between several of these
feedbacks, which explained a reduced overall aerosol indirect effect on
summertime precipitation over Germany. Although similar to our HR
simulations, they used day-by-day simulations and on a rather small domain,
which potentially prevents the long-term effects described by <xref ref-type="bibr" rid="bib1.bibx17" id="normal.25"/>
from being captured. Our simulation domain and duration are large enough for
such behaviors to be possibly observable.</p>
      <p id="d1e212">Among them, there is the aerosol cooling effect on the surface caused by
reduced solar energy reaching the surface with increased aerosol
concentrations. This cooling can be due to the direct effect of the aerosols
or to their indirect effects. Surface cooling due to aerosol effects and the
consecutive reduction of precipitation have been mostly described on the
global scale by studies such as <xref ref-type="bibr" rid="bib1.bibx53" id="text.26"/>, <xref ref-type="bibr" rid="bib1.bibx60" id="text.27"/>, <xref ref-type="bibr" rid="bib1.bibx7" id="text.28"/>,
and by <xref ref-type="bibr" rid="bib1.bibx29" id="text.29"/> for the Mediterranean area. On the cloud-resolving
scale, the effect on precipitation of the surface cooling due to the indirect
effect of aerosols has been studied by <xref ref-type="bibr" rid="bib1.bibx62" id="text.30"/> and <xref ref-type="bibr" rid="bib1.bibx17" id="text.31"/>.<?pagebreak page323?> Both of these
studies find a surface cooling due to the aerosol indirect effect, with weak
effects on precipitation in spite of the stabilization of the atmospheric
columns. <xref ref-type="bibr" rid="bib1.bibx38" id="text.32"/> examine the stabilization of the atmosphere due
to upper-tropospheric warming as a consequence of the aerosol indirect
effects, yielding a small reduction of precipitation. However, stabilization
of the atmospheric column does not always cause a reduction of precipitation,
since this effect is in competition with the invigoration effect discussed by
<xref ref-type="bibr" rid="bib1.bibx17" id="text.33"/>. This aerosol invigoration effect has been shown to potentially
enhance precipitation in certain conditions but cannot act on the global
overall amount of precipitation since it does not modify the evaporation
flux.</p>
      <p id="d1e240">Observational studies of these effects are hindered by the fact that
observations can not easily separate the aerosol indirect effects from other
effects <xref ref-type="bibr" rid="bib1.bibx9" id="paren.34"/>; therefore, global or regional models can be used for
this purpose. However, quite often, such studies are performed by changing
aerosol concentrations simultaneously in the radiative and microphysical
schemes of the model, which does not permit us to separate direct and indirect
effects from each other. This is the case for studies performed with high-resolution
models <xref ref-type="bibr" rid="bib1.bibx16 bib1.bibx31 bib1.bibx30 bib1.bibx36 bib1.bibx75" id="paren.35"/> or low-resolution
climate models <xref ref-type="bibr" rid="bib1.bibx35 bib1.bibx68 bib1.bibx22" id="paren.36"/>. In the present
study, as discussed above, we will use the model configurations to modulate
the aerosol indirect effects without affecting the aerosol direct effects.</p>
      <p id="d1e252">Section <xref ref-type="sec" rid="Ch1.S2"/> details the configuration of the WRF model used and
the simulations that have been performed for this sensitivity analysis.
Section <xref ref-type="sec" rid="Ch1.S3"/> analyses the sensitivity experiment in both the HR
and LR simulations, and compare their sensitivities to the change in CCN
concentration. Section <xref ref-type="sec" rid="Ch1.S4"/> discusses the results and proposes a
synthesis of the various processes and interrelations involved in the aerosol
indirect effects on the Mediterranean summer precipitation.</p>
</sec>
<sec id="Ch1.S2">
  <title>Model presentations and configurations</title>
      <p id="d1e267">The model used in this study is version 3.7.1 of the Weather Research and
Forecasting model (WRF). WRF is a non-hydrostatic limited-area model with
mass coordinate vertical discretization designed to serve both operational
and research needs <xref ref-type="bibr" rid="bib1.bibx65" id="paren.37"/>.
The WRF simulations presented here
have been performed with a 50 km (LR) and a 3.3 km (HR) horizontal
resolution and 33 vertical layers from the surface to 50 hPa, with about
8 levels in the lowest 1000 m of the atmosphere. The simulation domain is
shown in Fig. <xref ref-type="fig" rid="Ch1.F1"/>. The Global Forecast System (GFS) model
<xref ref-type="bibr" rid="bib1.bibx47" id="paren.38"/> provided the initial and lateral conditions updated every 6 h,
with a 1<inline-formula><mml:math id="M1" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> resolution in longitude and latitude. A Newtonian-type
nudging with relaxation towards GFS analysis data and a coefficient of <inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:mn mathvariant="normal">5</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> s<inline-formula><mml:math id="M3" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> has been applied for temperature, humidity,
geopotential, and velocity components, as recommended by <xref ref-type="bibr" rid="bib1.bibx59" id="text.39"/> and <xref ref-type="bibr" rid="bib1.bibx48 bib1.bibx49" id="text.40"/>.</p>
      <p id="d1e324">The sea surface temperature (SST) is provided by GFS. The geographical data
are from 5<inline-formula><mml:math id="M4" display="inline"><mml:msup><mml:mi/><mml:mo>′</mml:mo></mml:msup></mml:math></inline-formula> resolution United States Geophysical Survey data. Soil type is
based on a combination of the 10<inline-formula><mml:math id="M5" display="inline"><mml:msup><mml:mi/><mml:mo>′</mml:mo></mml:msup></mml:math></inline-formula> resolution, 17 category United Nations
Food and Agriculture Organization soil data and US State Soil Geographic
10<inline-formula><mml:math id="M6" display="inline"><mml:msup><mml:mi/><mml:mo>′</mml:mo></mml:msup></mml:math></inline-formula> soil data. The set of parameterizations used for these simulations
include the improved Mellor–Yamada closure scheme (MYNN;
<xref ref-type="bibr" rid="bib1.bibx43 bib1.bibx44 bib1.bibx45 bib1.bibx46" id="altparen.41"/>) for the boundary
layer. The surface layer is the revised Monin–Obukov scheme
<xref ref-type="bibr" rid="bib1.bibx23" id="paren.42"/>. The microphysics scheme is the most important for this
study. The new Thompson and Eidhammer “aerosol-aware” formulation
<xref ref-type="bibr" rid="bib1.bibx73" id="paren.43"/> has been chosen for its ability to explicitly represent
cloud droplet nucleation and ice activation by aerosols. The scheme gives
one-moment prediction (mass mixing ratio) for snow, and a hybrid
graupel–hail category and two-moment predictions (mass mixing ratio and
number concentration) for cloud water, cloud ice, rain, and aerosols. The
latter are divided into two categories depending on their capacity to serve
as CCN (“water friendly aerosol”, WFA) or ice nuclei (“ice friendly aerosol”,
IFA). During model integration, the
number of WFA (NWFA) and the number of IFA (NIFA) are advected and diffused
exactly as other scalars. Aerosol number concentration is initialized and
forced at domain boundaries by a climatology. For WFA, a virtual surface
emission flux is computed from the horizontal grid spacing and the initial
NWFA values to approximately balance the loss of WFA due to nucleation and
scavenging, as described in <xref ref-type="bibr" rid="bib1.bibx73" id="text.44"/>. No surface emissions are
applied for NIFA. The 2-D tendency field is added at each time step to the
first model vertical level NWFA value. The radiation scheme is RRTMG (rapid
radiative transfer model for general circulation models; <xref ref-type="bibr" rid="bib1.bibx21" id="altparen.45"/>),
which uses the correlated-<inline-formula><mml:math id="M7" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> approach to calculate longwave fluxes and
heating rates efficiently and accurately for application to global climate
models. We choose this scheme so that the microphysics scheme can communicate
cloud water droplets, ice, and snow effective radii to the radiation scheme,
which will then use these values to resolve the equations for radiative
transfer in each model column, providing quantities such as shortwave (SW)
and longwave (LW) radiative fluxes and the COD. It is important to note at
this point that the <xref ref-type="bibr" rid="bib1.bibx72" id="text.46"/> climatology provided to the RRTMG
radiative scheme will be unchanged when we perform sensitivity experiments by
modifying the microphysical NWFA and NIFA climatologies, which enables us to
modulate the indirect aerosol effect without changing the direct aerosol
effect.</p>
      <p id="d1e380">The convection is parameterized using the <xref ref-type="bibr" rid="bib1.bibx24" id="text.47"/> scheme. This scheme
triggers convection whenever a given atmospheric layer is diagnosed as
unstable, taking into<?pagebreak page324?> account its temperature and moisture, the temperature
gap between the adiabatically lifted atmospheric parcel and its environment
at its lowest condensation level (LCL), and the large-scale vertical wind
speed. If a given atmospheric layer (60 hPa thick) is diagnosed to be able
to reach its LCL given the above-mentioned parameters, then it is released at
this altitude with an initial vertical velocity of up to several meters per
second, depending on the atmospheric conditions. A Lagrangian parcel method
including entrainment, detrainment, and water loading is applied. If the
atmospheric parcel is able to raise by at least 3–4 km, convection is
triggered, and lasts until when the Convective Available Potential Energy
(CAPE) is consumed. It is worth noting that at that point the microphysical
effects of aerosols are not taken into account explicitly in this
parameterization. However, they can modulate the occurrence and intensity of
parameterized convection because they affect the background temperature and
moisture profiles through the above-mentioned indirect effects, taken into
account by the <xref ref-type="bibr" rid="bib1.bibx73" id="normal.48"/> scheme.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><caption><p id="d1e391">Simulation domain with gray-shaded area indicating a topography
higher than 500 m. The EUR and MED boxes indicate the regions that will be
used below. The Low Resolution domain is the entire map (LR) and the small
box inside the EUR box indicate the High Resolution domain
(HR).</p></caption>
        <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f01.png"/>

      </fig>

      <p id="d1e401">The model was run with two different NWFA and NIFA microphysical forcings for
6 months covering spring and summer 2013. The two simulations start on
1 April 2013 (after 1 month spin-up) and end on 30 September 2013. We
performed two “extreme” simulations in terms of NWFA and NIFA
concentrations. In the first simulation, hereafter referred to as MAX or
polluted simulation, a very high aerosol emission level is applied (<inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.75</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">7</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> kg s<inline-formula><mml:math id="M9" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the whole domain), whereas for the other
simulation, hereafter referred to as MIN or pristine simulation, a very low
aerosol emission level is applied (<inline-formula><mml:math id="M10" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.75</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> kg s<inline-formula><mml:math id="M11" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for
the whole domain). Although emission rates are extreme between MIN and MAX
simulations, the application of the microphysics scheme constrains the range
of variation in NWFA to be between <inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> cm<inline-formula><mml:math id="M13" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and
<inline-formula><mml:math id="M14" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> 000 cm<inline-formula><mml:math id="M15" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and of NIFA to be between 0.005 cm<inline-formula><mml:math id="M16" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and
10 000 cm<inline-formula><mml:math id="M17" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, so that the extreme emission rates imposed in the MAX and
MIN simulations only ensure that NIFA and NWFA concentrations in the MAX
(resp. MIN) simulation stay close to their maximal (resp. minimal) permitted
values, corresponding to a factor of <inline-formula><mml:math id="M18" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> for NWFA and <inline-formula><mml:math id="M19" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> for NIFA between the MAX and MIN simulations. These extreme values
ensure that aerosol indirect effects emerge from the “natural noise”
between MIN and MAX simulations. Except this difference in the NWFA and NIFA
concentrations between the MAX and MIN simulations, the configuration of both
simulations is strictly the same, so that all the observed differences
between the MAX and MIN simulations can be attributed to these different
concentrations of NIFA and NWFA.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><caption><p id="d1e563">Accumulated precipitation (April–September 2013) from the MIN
simulation <bold>(a)</bold> and difference between MAX and MIN simulations of
accumulated precipitation <bold>(b)</bold>. </p></caption>
        <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f02.png"/>

      </fig>

      <p id="d1e578">Apart from these two simulations on the LR domain, two companion simulations
have been performed at a convection-permitting resolution (3.3 km) on the HR
domain, which is a smaller domain (to keep computational cost under control)
shown on Fig. <xref ref-type="fig" rid="Ch1.F1"/>. The location of the domain was chosen far
from the oceans (to avoid sea contamination) and from the edges of the LR
domain (to avoid boundary condition contamination). One simulation on this
HR domain has been performed with maximal concentrations of NWFA and NIFA,
the other one with minimal concentrations. These simulations are forced at
their boundaries by the LR MAX and MIN simulations, respectively, through
one-way nesting, using an intermediate resolution domain at 16.6 km resolution,
also shown in Fig. <xref ref-type="fig" rid="Ch1.F1"/>. Due to these successive
increases in the resolution by a factor of 5 and then by a factor of 3, each grid
cell of the LR domain corresponds to exactly <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:mn mathvariant="normal">15</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">15</mml:mn></mml:mrow></mml:math></inline-formula> grid cells of the
HR domain. The configuration of the low-resolution and intermediate
resolution simulations is exactly the same. Regarding the high-resolution
simulations, the only difference in model configuration is that the
<xref ref-type="bibr" rid="bib1.bibx24" id="text.49"/> convection scheme is turned off since model horizontal
resolution becomes sufficient to explicitly resolve the convection processes.</p>
      <p id="d1e600">The analysis of the simulations will be conducted on two distinct sub-domains
in Europe (EUR) and the Mediterranean region (MED; see
Fig. <xref ref-type="fig" rid="Ch1.F1"/>). In the absence of an interactive ocean model, the
SST remains prescribed and is the same in both simulations. Therefore, the SST
is not in equilibrium with the heat fluxes at the air–sea interface, which is
the reason why we will focus all our analyses on atmospheric
columns above the continental surface in this study.</p>
</sec>
<sec id="Ch1.S3">
  <title>Sensitivity experiment analysis</title>
<sec id="Ch1.S3.SS1">
  <title>Sensitivity of the LR simulation to the CCN load</title>
      <p id="d1e616">Figure <xref ref-type="fig" rid="Ch1.F2"/> displays the geographical pattern of total
accumulated precipitation from the MIN simulation. Except for the
northeastern part of the Atlantic Ocean, summer precipitation is mostly
located over land, particularly over central and<?pagebreak page325?> eastern Europe as well as
over the main mountain ranges. Figure <xref ref-type="fig" rid="Ch1.F2"/> also shows the
total accumulated precipitation difference between MAX and MIN simulations
(MAX-MIN). Differences are ranging around 5–10 %. Such values are large
compared to those found in the study of <xref ref-type="bibr" rid="bib1.bibx73" id="text.50"/> with the same
model and microphysics scheme (the difference between their polluted and
clean simulations for a winter cyclone in the USA is 1.1 %). This is as
expected because in our study the ratio of aerosol concentrations between our
clean and polluted numerical experiments is much larger (<inline-formula><mml:math id="M21" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> vs. <inline-formula><mml:math id="M22" display="inline"><mml:mn mathvariant="normal">10</mml:mn></mml:math></inline-formula> in
<xref ref-type="bibr" rid="bib1.bibx73" id="altparen.51"/>). The pattern of accumulated precipitation
differences displays neighboring
dipoles of positive and negative differences, suggesting compensating effects
or shifts in the precipitation maxima.</p>
      <p id="d1e648">Let us first evaluate the first indirect aerosol effect and assess its
consequences on precipitation. Figure <xref ref-type="fig" rid="Ch1.F3"/> displays downward
surface SW, LW, and total radiation differences as a function of COD differences over the continental regions of
the EUR and MED domains. The COD is computed using the following simplified
equation:
            <disp-formula id="Ch1.E1" content-type="numbered"><mml:math id="M23" display="block"><mml:mrow><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>=</mml:mo><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mtext>LWC</mml:mtext><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>w</mml:mtext></mml:msub><mml:msub><mml:mi>R</mml:mi><mml:mi>e</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mtext>d</mml:mtext><mml:mi>z</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where LWC is the liquid water content, <inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ρ</mml:mi><mml:mtext>w</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> the water density, and
<inline-formula><mml:math id="M25" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>e</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the droplet radius, and the integral is performed from the surface to
the top of atmosphere (or, in our case, from the surface to the model top
which is at 50 hPa). Only results for cloud liquid water are shown as
results for ice are comparatively negligible. It shows that the effect of
this increased COD is twofold, reducing the downward SW radiative flux at the
surface (due to increased cloud albedo), but increasing the downward LW
radiation due to LW emissions by the optically thicker clouds. However, the
effect in the SW band largely dominates the effect in the LW band, leading in
our case to a radiative cooling proportional to the change in COD between
both simulations. The fact that the modifications of the SW flux dominate
those of the LW flux in our study is in line with the findings of
<xref ref-type="bibr" rid="bib1.bibx17" id="text.52"/> for the United States, China, and the tropical western Pacific. The
fact that the modifications of the SW flux dominate those of the LW flux
cannot be generalized to all conditions, since the comparison between these
two terms depend on several parameters such as the solar zenith angle,
surface albedo, cloud optical depth, and cloud altitude, as described by
<xref ref-type="bibr" rid="bib1.bibx54" id="text.53"/>, <xref ref-type="bibr" rid="bib1.bibx69" id="text.54"/>, <xref ref-type="bibr" rid="bib1.bibx1" id="text.55"/>, and <xref ref-type="bibr" rid="bib1.bibx64" id="text.56"/>.</p>
      <p id="d1e728">These results are a logical consequence of the Twomey effect, which tends to
increase the COD in the presence of stronger concentrations of WFA. On the
one side, the increase in the total cross section of cloud droplets leads to
higher cloud albedo and therefore to lower downward surface solar radiation.
On the other side, the larger the COD, the larger the LW radiation emission
by clouds. As discussed before, the difference in surface radiative heating
which accounts for both SW and LW radiations remains systematically negative
in our study.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><caption><p id="d1e733">Mean downward surface shortwave (<inline-formula><mml:math id="M26" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mtext>SW</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, black),
longwave (<inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mtext>LW</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, green), and total (<inline-formula><mml:math id="M28" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mtext>tot</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>,
red) radiation differences as a function of the mean COD difference (<inline-formula><mml:math id="M29" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="italic">τ</mml:mi></mml:mrow></mml:math></inline-formula>) over the EUR <bold>(a)</bold> and MED <bold>(b)</bold> domains.
</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f03.png"/>

        </fig>

      <p id="d1e799">Let us split total precipitation (<inline-formula><mml:math id="M30" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
into their explicit (i.e., large-scale; <inline-formula><mml:math id="M31" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">expl</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">expl</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and convective (i.e. parameterized; <inline-formula><mml:math id="M32" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) components.
Figure <xref ref-type="fig" rid="Ch1.F4"/> shows the relative difference between MAX
and MIN simulations of convective, explicit, and total precipitation over
continent as a function of the fraction of convective precipitation
(<inline-formula><mml:math id="M33" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) in the EUR and MED domains
(Fig. <xref ref-type="fig" rid="Ch1.F1"/>). At each grid point in each domain, the relative
differences in accumulated convective, explicit, and total precipitation are
paired with convective precipitation fraction. The pairs<?pagebreak page326?> are placed in bins
with an equal number of samples in each bin (50 samples) and therefore
varying ranges of convective precipitation fraction for each bin. For each
bin, the median convective precipitation fraction and median relative
precipitation difference are computed. Summer convective precipitation are
clearly weakened by the addition of aerosols, while it is the opposite for
large-scale precipitation. Similar results are obtained for low precipitation
rate (20th percentile) and high precipitation rate (80th percentile; not
shown), which therefore confirm the robustness of the results.
Figure <xref ref-type="fig" rid="Ch1.F4"/> suggests a compensating effect between
explicit and convective precipitation leading to a non-significant difference
for total accumulated precipitation. To explain this, a similar pair of
simulations have been performed without activating the convection scheme. The
analysis of these two simulations also confirm an increase in large-scale
precipitation when aerosol concentrations increase, thus discarding the
compensating effect (not shown). On the contrary, it suggests an independent
positive effect of aerosols on non-convective precipitation.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><caption><p id="d1e889">Relative difference between the MAX and MIN simulations of
continental summer convective (<inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
dotted), not convective (<inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">expl</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">expl</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, dashed),
and total (<inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, solid) accumulated
precipitation as a function of convective precipitation fraction
(<inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) over Europe (EUR domain,
Fig. <xref ref-type="fig" rid="Ch1.F1"/>) <bold>(a)</bold> and the Mediterranean region (MED
domain, Fig. <xref ref-type="fig" rid="Ch1.F1"/>) <bold>(b)</bold>. </p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f04.pdf"/>

        </fig>

      <p id="d1e987">Since 50–85 % of the radiative heating is balanced by evaporation
<xref ref-type="bibr" rid="bib1.bibx26" id="paren.57"/>, a correlated modification of low-level water vapor mixing
ratio should be observed. Figure <xref ref-type="fig" rid="Ch1.F5"/> displays the
relationship between the difference between MAX and MIN simulations of
convective precipitation (<inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and of surface water
mixing ratio (<inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow></mml:math></inline-formula>). For each grid points, the differences in hourly
convective precipitation (<inline-formula><mml:math id="M40" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are paired with the
difference of surface water mixing ratio (<inline-formula><mml:math id="M41" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow></mml:math></inline-formula>). The pairs are placed
in bins with an equal number of samples in each bin (20 000 samples). For
each bin, the median values are computed as well as the 20th and 80th
percentiles and are displayed in Fig. <xref ref-type="fig" rid="Ch1.F5"/>.
Figure <xref ref-type="fig" rid="Ch1.F5"/> shows that a decrease (increase) in surface water
mixing ratio is associated almost systematically with a decrease (increase)
in convective precipitation. Despite less local evaporation, some convective
events are characterized by higher available surface water vapor with an
associated increase in convective precipitation. The origin may be a
“contamination” by the sea. Indeed, since the SST is imposed and is not in
equilibrium with the reduction of downward solar radiation and because
evaporation flux at the surface of the sea is in part driven by the
temperature difference between the air and the sea surface (e.g.,
<xref ref-type="bibr" rid="bib1.bibx37" id="altparen.58"/>; on which the Unified NOAH Land Surface Model – which is used
in this study – is based), erroneous evaporation fluxes are expected to be
simulated over the sea.</p>
      <p id="d1e1049">In the coastal land of the Mediterranean region in summertime, sea breezes
advect marine moist air over a few tens of kilometers inland (e.g.,
<xref ref-type="bibr" rid="bib1.bibx4 bib1.bibx5 bib1.bibx11 bib1.bibx14" id="altparen.59"/>), which can cause inland
precipitation. The absence of air–sea feedbacks in this simulation therefore
affects inland humidity advection and convective precipitation in the coastal
areas (e.g., <xref ref-type="bibr" rid="bib1.bibx29 bib1.bibx28" id="altparen.60"/>).</p>
      <p id="d1e1058">In these simulations, aerosols reduce total precipitation through their
parameterized part. In order to check if this effect is not only a
parameterization effect, we performed a 3.3 km resolution simulation without
activating the convective scheme. The following part aims at determining if
the same precipitation reduction effect is also present in the
convection-permitting simulation.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><caption><p id="d1e1064">Difference between MAX and MIN simulations of convective
precipitation (<inline-formula><mml:math id="M42" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and of surface water mixing ratio
(<inline-formula><mml:math id="M43" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow></mml:math></inline-formula>) for EUR <bold>(a)</bold> and MED <bold>(b)</bold> domains. The thick
black line corresponds to the ensemble average. The lower and upper dotted
lines delimiting the shaded area are the 20th and 80th percentiles,
respectively. </p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f05.png"/>

        </fig>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><caption><p id="d1e1105">Comparison of precipitation statistics between LR and HR
simulations. Space-averaged temporal correlation for the hourly, daily, and
weekly precipitation amounts, respectively (first row); same for the
time-averaged spatial correlation (second row); accumulated precipitation
(mm) averaged over the HR domain from the whole LR and HR simulation time
series (third and fourth rows).</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MIN</oasis:entry>
         <oasis:entry colname="col3">MAX</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Temporal correlation HR–LR</oasis:entry>
         <oasis:entry colname="col2">0.38/0.60/0.72</oasis:entry>
         <oasis:entry colname="col3">0.31/0.54/0.69</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Spatial correlation HR–LR</oasis:entry>
         <oasis:entry colname="col2">0.32/0.52/0.68</oasis:entry>
         <oasis:entry colname="col3">0.28/0.46/0.62</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Accumulated precipitation LR (mm)</oasis:entry>
         <oasis:entry colname="col2">414</oasis:entry>
         <oasis:entry colname="col3">384</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Accumulated precipitation HR (mm)</oasis:entry>
         <oasis:entry colname="col2">305</oasis:entry>
         <oasis:entry colname="col3">272</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S3.SS2">
  <?xmltex \opttitle{Sensitivity of the HR simulations and impact\hack{\break} of the resolution}?><title>Sensitivity of the HR simulations and impact<?xmltex \hack{\break}?> of the resolution</title>
      <p id="d1e1193">At this point, it is suitable to check how the LR simulation behaves in terms
of precipitation amount, localization, and timing compared to the
convection-permitting HR simulation. Figure <xref ref-type="fig" rid="Ch1.F6"/> shows daily
MIN time series of precipitation for a LR grid point that is inside the HR
domain. HR precipitation time series were made considering the average of the
<inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:mn mathvariant="normal">15</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">15</mml:mn></mml:mrow></mml:math></inline-formula> grid cell that are inside the LR grid cell. This time series
shows that the LR simulation is able to reproduce the main features of the HR
simulation, including the succession of long-lasting rainy and dry sequences,
as well as the occurrence of precipitation maxima for individual days,<?pagebreak page327?> even
though some of these peaks are stronger in the LR simulation than in the HR
simulation or conversely. Table <xref ref-type="table" rid="Ch1.T1"/> shows a comparison of temporal
and spatial statistics of precipitation between the LR and HR simulations. In the
first line we can see the spatial average of the hourly, daily, and weekly
correlations of precipitation amounts between LR and HR simulations,
performed by first calculating the correlation of the hourly (resp. daily,
weekly) precipitation amount between each of the cells of the LR model vs.
the corresponding precipitation amount for the <inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:mn mathvariant="normal">15</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">15</mml:mn></mml:mrow></mml:math></inline-formula> matching cells
of the HR domain, and then averaging all these local time correlations over
the whole intersection of the HR and LR domains.</p>
      <p id="d1e1224">One can note a correlation around 0.3 in both MIN and MAX simulations on the
hourly timescale between the LR and the HR simulations. The correlation
coefficient increases for longer timescales, reaching 0.57 on daily timescale
and around 0.71 on weekly timescale for both MAX and MIN simulations, which
shows that even though the LR simulation does not succeed in having the
precipitation events with exactly the same timing and intensity as in the HR
simulation, these differences tend to be strongly reduced on the weekly timescale,
which is satisfying since RCMs are usually used for climate studies.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><caption><p id="d1e1229">Daily MIN precipitation time series for the LR (blue) and HR (red)
simulations in one LR grid cell located close to the center of the HR domain.
</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f06.png"/>

        </fig>

      <p id="d1e1239">Let us now evaluate the spatial distribution of precipitation in the LR
simulation. Figure <xref ref-type="fig" rid="Ch1.F7"/> displays the MIN hourly
cumulated precipitation for the day of 12 May 2013 in the HR domain, for the
HR simulation (top left), the LR simulation (top right), and for the HR
precipitation aggregated on the LR grid by averaging on each LR grid cell the
<inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:mn mathvariant="normal">15</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">15</mml:mn></mml:mrow></mml:math></inline-formula> matching HR grid cells (bottom right). We can see that the spatial
distributions of the HR and LR simulations are rather similar on a large scale,
even though the precipitation tends to be spread over larger areas in the LR
simulation than in the HR simulation, even after aggregation of the latter on
the LR grid, with a corresponding reduction of the maximal values of
precipitation rates in the LR simulation.</p>
      <p id="d1e1256">As seen in the second line of Table <xref ref-type="table" rid="Ch1.T1"/>, averaged spatial
correlation increases from around 0.30 on an hourly timescale to around 0.65
on a weekly timescale for both MIN and MAX simulations. Similarly, averaged
spatial correlations increase when we cluster grid points (not shown). It shows that even if precipitation is
not exactly located at the same grid point and at the right time, spatial
patterns are globally respected as seen in our example
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>). Therefore, as for the temporal
correlations, the examination of spatial correlations shows that the spatial
agreement between the HR and LR becomes satisfactory when the analysis is
focused on daily or weekly timescales, which once again is in line with the
typical uses of long-term RCM simulations.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><caption><p id="d1e1265">Precipitation amount (in mm) between 13:00 and 14:00 UTC on
12 May 2013 for the MIN HR simulation <bold>(a)</bold>, MIN LR
simulation <bold>(b)</bold> and the HR simulation aggregated on the LR grid by
averaging on each LR grid cell the <inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:mn mathvariant="normal">15</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">15</mml:mn></mml:mrow></mml:math></inline-formula> matching HR grid
cells <bold>(c)</bold>.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f07.png"/>

        </fig>

      <p id="d1e1295">A comparison of the accumulated precipitation over the whole HR domain for the
entire 6 months of simulation between the HR and LR simulations
(Table <xref ref-type="table" rid="Ch1.T1"/>) reveals that the accumulated precipitation in the LR
simulation is significantly stronger than in the HR simulation, both for the
MIN and MAX experiments. However, the indirect effect of aerosols on the
precipitation is similar in the LR simulation than in the HR simulation
(<inline-formula><mml:math id="M48" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>11 % in the HR simulation and <inline-formula><mml:math id="M49" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7 % in the LR simulation). This
shows that even though the LR simulation with the Kain–Fritsch convection
scheme simulates stronger precipitation than the convection-permitting HR
simulation, the microphysical effects of aerosols on precipitation in the LR
simulation are of the same sign and magnitude than in the HR simulation,
which tends to strengthen the results presented for the LR simulation in
Sect. <xref ref-type="sec" rid="Ch1.S3.SS1"/>.</p>
</sec>
</sec>
<?pagebreak page328?><sec id="Ch1.S4">
  <title>Discussion</title>
      <p id="d1e1323">Table <xref ref-type="table" rid="Ch1.T2"/> displays various key variables averaged over all of the
simulation period and over the EUR and MED domains. By examining the
sensitivity of these key variables to the CCN load in both the HR and LR
simulations, we will try to discuss the plausible processes involved in the
simulated reduction of precipitation due to the aerosol indirect effects,
which we sum up in Fig. <xref ref-type="fig" rid="Ch1.F8"/> – a summary of most of the
effects discussed in the present study.</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T2"><caption><p id="d1e1333">Key variables for the MIN and MAX simulations: number of cloud
condensation nuclei (NCCN), number of liquid cloud drops
(<inline-formula><mml:math id="M50" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">drops</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), liquid water content (LWC), cloud drops effective radii
(<inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), cloud optical depth (COD), shortwave downward radiations
(SWD), longwave downward radiations (LWD), latent heating (LH), surface
temperature (<inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">surf</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), surface water vapor mixing ratio
(<inline-formula><mml:math id="M53" display="inline"><mml:mrow><mml:msub><mml:mi>Q</mml:mi><mml:mi mathvariant="normal">surf</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), number of hours per grid point with strictly positive
MuCAPE (<inline-formula><mml:math id="M54" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">hour</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> MuCAPE), MuCAPE, MuCIN, convective precipitation
(<inline-formula><mml:math id="M55" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and total precipitation (<inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). All the
values are averaged in space and time over the indicated domain from April to
September 2013, except <inline-formula><mml:math id="M57" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M58" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (precipitation
totals averaged over space only) and <inline-formula><mml:math id="M59" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">hour</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> MuCAPE (number of
hours averaged over space only).</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.85}[.85]?><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Field</oasis:entry>
         <oasis:entry colname="col2">Box</oasis:entry>
         <oasis:entry colname="col3">MIN</oasis:entry>
         <oasis:entry colname="col4">MAX</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M60" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mi mathvariant="normal">MAX</mml:mi><mml:mo>-</mml:mo><mml:mi mathvariant="normal">MIN</mml:mi></mml:mrow><mml:mi mathvariant="normal">MIN</mml:mi></mml:mfrac></mml:mstyle></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">NCCN (no. cm<inline-formula><mml:math id="M61" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">12.9</oasis:entry>
         <oasis:entry colname="col4">10 631</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M62" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>823</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">13.6</oasis:entry>
         <oasis:entry colname="col4">16 226</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M63" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1192</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">14.5</oasis:entry>
         <oasis:entry colname="col4">9321</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M64" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>642</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">drops</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (no. cm<inline-formula><mml:math id="M66" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">1.13</oasis:entry>
         <oasis:entry colname="col4">58.6</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M67" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>50.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">0.80</oasis:entry>
         <oasis:entry colname="col4">33.4</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M68" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>40.8</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">6.3</oasis:entry>
         <oasis:entry colname="col4">267</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M69" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>41.4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LWC (<inline-formula><mml:math id="M70" display="inline"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">11</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> kg cm<inline-formula><mml:math id="M71" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">2.1</oasis:entry>
         <oasis:entry colname="col4">6.1</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M72" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">1.4</oasis:entry>
         <oasis:entry colname="col4">3.2</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M73" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.3</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">9.1</oasis:entry>
         <oasis:entry colname="col4">16.2</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M74" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.78</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M75" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">eff</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M76" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">16.0</oasis:entry>
         <oasis:entry colname="col4">6.2</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M77" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.61</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">14.7</oasis:entry>
         <oasis:entry colname="col4">6.1</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M78" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.59</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">14.4</oasis:entry>
         <oasis:entry colname="col4">5.5</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M79" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.62</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">COD</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">0.56</oasis:entry>
         <oasis:entry colname="col4">3.6</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M80" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>5.4</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">0.20</oasis:entry>
         <oasis:entry colname="col4">0.98</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M81" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.9</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">1.09</oasis:entry>
         <oasis:entry colname="col4">6.20</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M82" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">SWD (W m<inline-formula><mml:math id="M83" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">292</oasis:entry>
         <oasis:entry colname="col4">276</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M84" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.05</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">330</oasis:entry>
         <oasis:entry colname="col4">325</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M85" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.01</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">283</oasis:entry>
         <oasis:entry colname="col4">266</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M86" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.06</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LWD (W m<inline-formula><mml:math id="M87" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">308</oasis:entry>
         <oasis:entry colname="col4">310</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M88" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.008</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">312</oasis:entry>
         <oasis:entry colname="col4">312</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M89" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.001</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">319</oasis:entry>
         <oasis:entry colname="col4">320</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M90" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.003</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LH (W m<inline-formula><mml:math id="M91" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">53.1</oasis:entry>
         <oasis:entry colname="col4">50.1</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M92" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.056</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">28.7</oasis:entry>
         <oasis:entry colname="col4">27.9</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M93" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.028</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">50.5</oasis:entry>
         <oasis:entry colname="col4">46.5</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M94" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.079</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M95" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">surf</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (K)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">290.2</oasis:entry>
         <oasis:entry colname="col4">289.6</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M96" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.002</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">295.1</oasis:entry>
         <oasis:entry colname="col4">294.9</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M97" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.001</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">289.7</oasis:entry>
         <oasis:entry colname="col4">289.0</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M98" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.002</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M99" display="inline"><mml:mrow><mml:msub><mml:mi>Q</mml:mi><mml:mi mathvariant="normal">surf</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (g kg<inline-formula><mml:math id="M100" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">6.63</oasis:entry>
         <oasis:entry colname="col4">6.58</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M101" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.008</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">5.82</oasis:entry>
         <oasis:entry colname="col4">5.83</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M102" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.002</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">6.47</oasis:entry>
         <oasis:entry colname="col4">6.37</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M103" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.015</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">hour</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> MuCAPE</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">1823</oasis:entry>
         <oasis:entry colname="col4">1830</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M105" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.004</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">771</oasis:entry>
         <oasis:entry colname="col4">760</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M106" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.01</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">1869</oasis:entry>
         <oasis:entry colname="col4">1804</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M107" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.03</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MuCAPE (J kg<inline-formula><mml:math id="M108" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">173</oasis:entry>
         <oasis:entry colname="col4">159</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M109" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.08</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">160</oasis:entry>
         <oasis:entry colname="col4">150</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M110" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.06</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">183</oasis:entry>
         <oasis:entry colname="col4">148</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M111" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.19</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MuCIN (J kg<inline-formula><mml:math id="M112" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">21.5</oasis:entry>
         <oasis:entry colname="col4">20.3</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M113" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.06</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">29.9</oasis:entry>
         <oasis:entry colname="col4">28.7</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M114" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.04</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">23.3</oasis:entry>
         <oasis:entry colname="col4">19.6</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M115" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.16</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M116" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">conv</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (mm)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">159</oasis:entry>
         <oasis:entry colname="col4">133</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M117" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.16</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">57</oasis:entry>
         <oasis:entry colname="col4">50</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M118" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.12</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M119" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">tot</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (mm)</oasis:entry>
         <oasis:entry colname="col2">EUR</oasis:entry>
         <oasis:entry colname="col3">322</oasis:entry>
         <oasis:entry colname="col4">306</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M120" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.05</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">MED</oasis:entry>
         <oasis:entry colname="col3">91</oasis:entry>
         <oasis:entry colname="col4">84</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M121" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.08</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">HR</oasis:entry>
         <oasis:entry colname="col3">305</oasis:entry>
         <oasis:entry colname="col4">272</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M122" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.11</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

      <p id="d1e2735">The ratio of CCN between the MIN and MAX simulations is about 1000, with no
major difference between the EUR and MED domains as the forcing climatology
is uniform over the whole domain. In detail, the NCCN is larger in the MED
region in spite of the identical forcing emissions since a smaller NCCN is
used for condensation, and wet scavenging of CCN
is less active due to the weak amount of precipitation
(Fig. <xref ref-type="fig" rid="Ch1.F2"/>a). As expected, the number of liquid cloud
droplets (Ndrops) increases massively with increasing aerosol concentration
(this number is multiplied by 40 to 50 between the MIN and MAX experiment in
the three examined simulation pairs). One can note that the relative
difference in Ndrops is smaller than that of NCCN as only a fraction of
aerosols is used for condensation, especially in the MAX simulation in which
the number of aerosols does not limit the condensation of the available
water. An increase in the number of droplets due to increased availability of
CCN is the first step in the process relating the increase in aerosol
concentration to the reduction of convective precipitation as shown in
Fig. <xref ref-type="fig" rid="Ch1.F8"/>. This larger number of droplets is associated
with smaller droplet radius (Reff) as a given amount of water is distributed
over more droplets (Table <xref ref-type="table" rid="Ch1.T2"/> and Fig. <xref ref-type="fig" rid="Ch1.F8"/>). The
relative difference between the MAX and MIN simulations of the droplet radii
is significant and on average equal to <inline-formula><mml:math id="M123" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>60 %.</p>
      <p id="d1e2753">Table <xref ref-type="table" rid="Ch1.T2"/> also shows that the available amount of water is sensitive
to the aerosol load, with an increase in the liquid water content (LWC) in
the MAX experiment by about 78 to 190 % in the three simulation pairs. An
increase in the cloud lifetime in the MAX simulation might be the main
explanation (<xref ref-type="bibr" rid="bib1.bibx77 bib1.bibx2 bib1.bibx56" id="altparen.61"/>). However, on the one
hand, the aerosol cloud lifetime effect has been challenged in recent studies
(<xref ref-type="bibr" rid="bib1.bibx66 bib1.bibx63" id="altparen.62"/>), and on the other hand, even if this effect stands in
reality, it is not sure that our model is able to correctly simulate it since
the representation of entrainment and droplet evaporation has been showen to
be poor in parameterized models <xref ref-type="bibr" rid="bib1.bibx79" id="paren.63"/>.</p>
      <p id="d1e2768">Equation (1) shows that the COD is proportional to the LWC and inversely
proportional to the droplet radius. Therefore, the increase in the COD
between the MIN and MAX experiments (COD is multiplied by 4.9 up to 6.4 in
the three simulation pairs) is in part due to the increase in the LWC, and in
part due to the diminished droplet radius, these two effects being of similar
magnitude in our simulations. As a consequence of a massive increase in the
COD, the surface downward shortwave radiation (SWD) is reduced by about <inline-formula><mml:math id="M124" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1
to <inline-formula><mml:math id="M125" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>6 % (Table <xref ref-type="table" rid="Ch1.T2"/> and Fig. <xref ref-type="fig" rid="Ch1.F8"/>).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><caption><p id="d1e2791">Schematic summary of the proposed aerosol causal chain sequence for
the indirect effect of aerosols on convective precipitation
</p></caption>
        <?xmltex \igopts{width=298.753937pt}?><graphic xlink:href="https://angeo.copernicus.org/articles/36/321/2018/angeo-36-321-2018-f08.pdf"/>

      </fig>

      <p id="d1e2800">The decrease in SWD implies a decrease in the surface temperature
(Table <xref ref-type="table" rid="Ch1.T2"/>) with the same order of magnitude (<inline-formula><mml:math id="M126" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.2 to <inline-formula><mml:math id="M127" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.6 K)
as in <xref ref-type="bibr" rid="bib1.bibx62" id="normal.64"/> in Germany. The combination of SWD decrease and
surface temperature<?pagebreak page329?> decrease sum up to cause a decrease in surface
evaporation (LH) by about 3 to 6 % due to the smaller quantity of energy
available for evaporation and to the reduced capacity of the colder air to
transport water vapor (Clausius–Clapeyron law). A consequence is the
reduction of the surface water vapor mixing ratio. On average, it is the case over
the EUR domain (<inline-formula><mml:math id="M128" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.8 %) but not over the MED domain (<inline-formula><mml:math id="M129" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.2 %) due
to the “sea contamination” (prescribed sea surface temperature; Table <xref ref-type="table" rid="Ch1.T2"/>).
A reduced surface water vapor mixing ratio is
associated with reduced convective precipitation (Fig. <xref ref-type="fig" rid="Ch1.F5"/>;
with the exception of the contaminated coastal convective precipitation). The
reduction of precipitable water (increase in LWC does not compensate the
decrease in water vapor) available for convection partly inhibits convective
precipitation (Fig. <xref ref-type="fig" rid="Ch1.F8"/>). The terms Most unstable
Convective Available Potential Energy (MuCAPE) and Most unstable Convective
Inhibition (MuCIN) have been chosen to characterize the stability of the
atmosphere. MuCAPE represents the total amount of potential energy available
to the most unstable parcel of the atmospheric column while being lifted to
its level of free convection, and MuCIN represents the energy barrier needed for this
parcel to reach its level of free convection. By construction, the MuCAPE
parameter is always positive. Therefore, the difference in MuCAPE between
both simulations can only be non-zero when there is a potentially unstable
layer in at least one of the simulations. MuCAPE differences between both
simulations at a given time and place can reveal very diverse situations. If,
on one hand, <inline-formula><mml:math id="M130" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MIN</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M131" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MAX</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>, there is a potentially unstable
atmospheric layer in the MIN simulation but not in the MAX simulation (and
conversely). If, on the other hand, <inline-formula><mml:math id="M132" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MIN</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M133" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MAX</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>, then the atmospheric column is potentially unstable in both
simulations, and <inline-formula><mml:math id="M134" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MIN</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mtext>MuCAPE</mml:mtext><mml:mtext>MAX</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>
describes the difference in the potential intensity of convection between
both simulations.</p>
      <p id="d1e2922">To only analyze the potential intensity of the convection, we averaged values
of <inline-formula><mml:math id="M135" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MIN</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="normal">MuCAPE</mml:mi><mml:mtext>MAX</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> when both
energies are non-zero (which makes a sample of about 2.4 million hours spread
over 1499 grid points in the EUR domain and about 1.1 million hours spread
over 1606 grid points in the MED domain).</p>
      <p id="d1e2943">On the other hand, MuCIN is defined only when a level of free convection
exists, i.e., only when MuCAPE is strictly positive. For all these reasons, we
averaged MuCAPE and MuCIN considering only the events with strictly positive
MuCAPE in both simulations. Because of increased relative humidity, MuCIN is
reduced by about 4 to 6 % in the LR simulations, and up to 16 % in
the HR simulation. MuCAPE is also weaker by 6 to 8 % in the LR domain,
and up to 19 % for the HR simulation, mostly due to the lack of water
vapor and to lower surface temperatures. When convection is actually
triggered, this reduced MuCAPE induces weaker convective updraft and
therefore weaker convective precipitation. This reduction in convective
precipitation (Fig. <xref ref-type="fig" rid="Ch1.F8"/>) is of 16 % in the EUR domain,
and 12 % in the MED domain, and causes a reduction in total precipitation
of 5 to 8 % in the EUR and MED domains of the LR simulation, and 11 %
in the HR simulation (Table <xref ref-type="table" rid="Ch1.T2"/>).</p>
      <?pagebreak page330?><p id="d1e2951">The effect of the stabilization of the atmospheric columns due to the
indirect effect of the aerosols has already been examined by
<xref ref-type="bibr" rid="bib1.bibx38" id="text.65"/>, <xref ref-type="bibr" rid="bib1.bibx62" id="text.66"/>, and <xref ref-type="bibr" rid="bib1.bibx17" id="text.67"/>. While
<xref ref-type="bibr" rid="bib1.bibx38" id="text.68"/> find small reductions in the precipitation amounts due to
this stabilization, <xref ref-type="bibr" rid="bib1.bibx62" id="text.69"/> and <xref ref-type="bibr" rid="bib1.bibx17" id="text.70"/> find a slight
increase in precipitation in a polluted atmosphere, due to the convective
invigoration linked to increased ice formation in the upper troposphere, an
effect that cannot be represented in our LR simulation since the Kain–Fritsch
convective scheme we use here does not explicitly take into account the
effect of aerosols and nucleation. While it can be represented by our HR
simulation, it does not appear to play a dominant role in the conditions of
our study.</p>
</sec>
<sec id="Ch1.S5" sec-type="conclusions">
  <title>Conclusion</title>
      <p id="d1e2980">Aerosols affect atmospheric dynamics and precipitation through their direct
and semi-direct radiative effects as well as through their indirect effects.
In this study, we investigated the indirect effects of aerosols on summer
precipitation in the Euro-Mediterranean region. While it is difficult to
disentangle the indirect effects of aerosols from the direct and semi-direct
effects in reality, we have carried out a numerical sensitivity experiment
using the WRF model, which allows us to isolate indirect effects, all other
things being equal, while introducing uncertainties linked to the model
formulation.
Very large and unrealistic
perturbations were chosen in order to allow the indirect effect of aerosols to emerge
from these uncertainties. For this purpose, the Thompson aerosol-aware
microphysics scheme has been used in a pair of simulations run at 50 km
resolution for the spring and summer of 2013 (April–September) with extremely
high and low aerosol concentrations, respectively. The outputs of these
simulations have been analyzed in two areas, one over continental northern
Europe and the other for the continental areas of the Mediterranean basin
(Fig. 1). In order to strengthen the results obtained on precipitation with
this first set of simulations, we performed an additional pair of simulations
at a convection-permitting resolution (3.3 km) for a continental subdomain.</p>
      <p id="d1e2983">Analysis of the LR simulation
outputs has revealed two opposite responses to this increase in aerosols
concentrations. In the polluted simulation, the amount of convective
(parameterized) precipitation is reduced in comparison to the pristine
simulation (Fig. <xref ref-type="fig" rid="Ch1.F4"/>). The total precipitation is also
reduced, even though an increase in stratiform precipitation partly
compensates the reduction of convective precipitation (Table <xref ref-type="table" rid="Ch1.T2"/>).
An examination of the differences in several relevant variables between the
pristine and polluted simulation reveals that the polluted simulation has
more water droplets than the pristine simulation, and that these water
droplets tend to be smaller (Table <xref ref-type="table" rid="Ch1.T2"/>). Additionally, the liquid
water content of the atmosphere is also generally increased in the polluted
simulation (Table <xref ref-type="table" rid="Ch1.T2"/>), probably in part because the smaller
droplets tend to stay longer in the atmosphere before precipitating. Both the
quantity and the size effect contribute to an increase in the COD, and a
subsequent reduction in the SWD flux at the surface, which is only partly
compensated<?pagebreak page331?> by a much smaller increase in the net longwave radiative flux
(Fig. <xref ref-type="fig" rid="Ch1.F3"/> and Table <xref ref-type="table" rid="Ch1.T2"/>). The reduction of radiative
heating at the surface has consequences on the atmospheric stability through
a reduced evaporation and lower surface temperature in the polluted
simulation (Table <xref ref-type="table" rid="Ch1.T2"/>). The reduced evaporation leads to a lower
surface water vapor mixing ratio in the polluted simulation
(Fig. <xref ref-type="fig" rid="Ch1.F5"/> and Table <xref ref-type="table" rid="Ch1.T2"/>) that accounts not only for
the reduction of potential energy for convection (Table <xref ref-type="table" rid="Ch1.T2"/>) but
also the reduction of precipitable water. The increase in stability and the
reduction of surface water vapor content contributes to the reduction of
convective precipitation in the polluted simulation (Table <xref ref-type="table" rid="Ch1.T2"/>). A
visual summary of this causal chain has been presented in
Fig. <xref ref-type="fig" rid="Ch1.F8"/>. In these simulations with parameterized
convection, the stratiform (explicitly resolved) precipitation increase
partly compensates the decrease in convective (parameterized)
precipitation. Since it could be
envisioned that this increase in stratiform precipitation could just be a
consequence of the reduction of convective precipitation, for example through
a greater availability of water for stratiform precipitation due to reduced
convective rainfall, we performed an additional pair of pristine and polluted
simulations at the same resolution but without activating the convection
scheme. Analysis of these simulations has shown that an increase in
stratiform precipitation also occurs in this additional pair of simulations
where parameterized convection is turned off, thereby excluding the
hypothesis that the increase in stratiform precipitation is just an effect of
decreased convective precipitation. Therefore, the reasons for this increase
in large-scale precipitation in the polluted case remains an open question.</p>
      <p id="d1e3012">In order to confirm and strengthen this result of a net reduction of total
precipitation due to aerosol secondary effect in a regional climate model, at
least in the study area, and to show that this result is not just a
consequence of the choice of a particular scheme for parameterized convection
(in our case the Kain-Fritsch scheme), we analyzed the same variables as in
the low-resolution simulation in the pair of convection-permitting
simulations. Even though differences exist between the behavior of the
convection-permitting simulation pair compared to its large-scale
counterpart, the main features are similar to those of the large-scale
simulations: a strong increase in the number of cloud droplets and their liquid
water content in the polluted simulation compared to the pristine simulation,
a strong decrease in their size, a decrease in the SWD radiative flux, a decrease
of the surface temperature and surface humidity, and a marked decrease in the
MuCAPE, yielding an overall reduction of total precipitation during the
simulation period (Table <xref ref-type="table" rid="Ch1.T2"/>). Convective invigoration, which
numerically can not occur in LR simulations because the cumulus scheme is
insensitive to the aerosol concentration, actually may not be important in
the convection-permitting simulation either. This result was expected since
it has been shown that this invigoration effect is stronger in weak wind
shear and warm cloud-bases (<inline-formula><mml:math id="M136" display="inline"><mml:mo lspace="0mm">&gt;</mml:mo></mml:math></inline-formula> 15 <inline-formula><mml:math id="M137" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C) conditions
<xref ref-type="bibr" rid="bib1.bibx32 bib1.bibx15" id="paren.71"/>, which may not be the situations that occur most often
in mid-latitude regions. <xref ref-type="bibr" rid="bib1.bibx58" id="text.72"/> evaluated the amplitude of the
invigoration effect as a function of the CCN concentration. They claimed that
the weight of the parcel condensate increases with CCN concentration since
aerosols tend to suppress precipitation by the Albrecht effect. The increasing
weight of parcels with CCN load tends to counteract the release of more
freezing latent heating (due to invigoration effect) with increasing CCN.
They stated the existence of an optimal CCN concentration at 1200 cm<inline-formula><mml:math id="M138" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
for the strongest invigoration effect. Beyond this optimal CCN concentration
value, the invigoration effect tends to be weakened by the increasing weight
of parcels. The effect is even negative when reaching extreme values such
as 10 000 cm<inline-formula><mml:math id="M139" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which is the typical order of magnitude of our MAX
simulation (see Table <xref ref-type="table" rid="Ch1.T2"/>). This is another possible explanation
for the weak invigoration effect observed in our simulations.</p>
      <p id="d1e3066">Even though the reduction of precipitation occurs through their parameterized
part, the fact that the reduction of the total precipitation amount persists
in a high-resolution convection-permitting simulation, at least in the
central Europe domain used, suggests that this impact of indirect aerosol
effects on precipitation is not just a consequence of the formulation of the
convection scheme but reflects underlying physical processes for which we
propose a summary under the form of a causal chain
(Fig. <xref ref-type="fig" rid="Ch1.F8"/>).</p>
      <p id="d1e3072">The magnitude of the simulated impact of the secondary aerosol effects on
precipitation is estimated as a reduction of total precipitation by 5 to
11 % in our simulations, but since these simulations have been performed
with extremely low or extremely high concentrations of CCN, these values need
to be interpreted as an upper bound of the magnitude of this effect rather
than as a realistic estimate. Our result can also be seen as a buffered
response of atmosphere to the aerosol indirect forcing as mentioned in
<xref ref-type="bibr" rid="bib1.bibx70" id="text.73"/>. Indeed, analysis of the LR simulation shows that
stratiform clouds act in two opposite ways for surface precipitation in a
polluted environment: in a direct way they produce more stratiform rain, and
in an indirect way they decrease convective rain through their stabilization
effect. This compensation explains why extreme changes in aerosol concentrations produce only small changes in
total precipitation. If all of the mentioned aerosol indirect effects have
already been discussed in past studies, in particular those of
<xref ref-type="bibr" rid="bib1.bibx62" id="text.74"/> and <xref ref-type="bibr" rid="bib1.bibx17" id="text.75"/>, the present study makes it possible to
analyze which effects are dominant for summertime in the Euro-Mediterranean
area with a regional simulation, and comparing a low-resolution simulation
with parameterized convection to a cloud-resolving simulation. Compared to
studies such as the ones of <xref ref-type="bibr" rid="bib1.bibx38" id="text.76"/>, <xref ref-type="bibr" rid="bib1.bibx62" id="text.77"/>, and
<xref ref-type="bibr" rid="bib1.bibx17" id="text.78"/>, our study permits us to observe this effect in the same region
and period with these two different model configurations, showing that a
model configuration with parameterized convection can represent precipitation
reduction due to stabilization related to<?pagebreak page332?> the indirect effect of aerosols in
a way that is very similar to a cloud-resolving simulation. Therefore, the
present study suggests that, for the mid-latitudes in summertime, global or
regional climate models with parameterized convection may be able to capture
the precipitation changes due to the effect of radiative cooling by the
aerosol indirect effect in a realistic way, at least when compared to similar
models in a convection-permitting configuration over the same area. Using
such configurations with parameterized convections also permits us to clearly
separate the processes affecting stratiform precipitation from the ones
affecting convective precipitation, as we have done above.</p>
      <p id="d1e3094">Because of the time of computation, our high-resolution domain is rather
small, which would limit the physical interpretation to that selected area.
However, the typical scale of the precipitation difference patterns in
Fig. <xref ref-type="fig" rid="Ch1.F2"/> is less than half the size of the
HR domain,
so that the differences observed in the HR domain do not
reflect only a particular case of positive or negative effect on
precipitation but a reasonable sample of continental Europe. Of course, for
future studies, it would be interesting to have such a high-resolution study
for an entire continental-scale domain.</p>
      <p id="d1e3099">To strengthen the analysis of these processes and evaluate in a more
realistic way their magnitude, it will be necessary to perform simulations
with models that are able to take into account realistic aerosol levels as
well as their variations in space and time, which will be possible in
particular through the use of online-coupled models that treat aerosol
emission and transport in a realistic way, such as described in
<xref ref-type="bibr" rid="bib1.bibx3" id="text.79"/>. Also, our study was not able to examine these effects
over oceanic surfaces since the forcing by fixed SSTs that are not in
equilibrium with the perturbed atmospheric forcings does not permit to obtain
meaningful results over the oceans; this could be overcome by using models
which are coupled with an oceanic model. Finally, to resolve the full
lifetime of clouds and water vapor in the atmosphere, it would also be useful
to use a larger domain (global or hemispheric).</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability">

      <p id="d1e3109">The data used in this study are available upon request to
the authors.</p>
  </notes><notes notes-type="competinginterests">

      <p id="d1e3115">The authors declare that they have no conflict of
interest.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e3121">This work is a contribution to the HyMeX program (HYdrological cycle in the
Mediterranean EXperiment) through INSU-MISTRALS support. This research has
received funding from the French National Research Agency (ANR) project
REMEMBER (contract ANR-12-SENV-001).<?xmltex \hack{\newline}?><?xmltex \hack{\hspace*{4mm}}?> The
topical editor, Marc Salzmann, thanks two anonymous referees for help in
evaluating this paper.</p></ack><ref-list>
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<abstract-html><p>Aerosols affect atmospheric dynamics through their direct and
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and low aerosol concentrations.
An additional pair of simulations has been
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effects without the use of parameterized convection.</p><p>While the reduced radiative flux due to the direct effects of the aerosols is
already known to reduce precipitation amounts, there is still no general
agreement on the sign and magnitude of the aerosol indirect
forcing effect on precipitation,
with various processes competing with each other. Although some processes
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that links the aerosol effects on microphysics to their simulated effect on
precipitation, essentially through reduction of the radiative heating of the
surface and corresponding reductions of surface temperature, resulting in
increased atmospheric stability in the presence of high aerosol loads.</p></abstract-html>
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